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Activation and catalytic reactions of saturated hydrocarbons in the presence of metal complexes

Author: A E Shilov; G B Shulʹpin
Publisher: Dordrecht ; Boston : Kluwer Academic Publishers, 2000.
Series: Catalysis by metal complexes, v. 21.
Edition/Format:   eBook : Document : EnglishView all editions and formats
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Genre/Form: Electronic books
Additional Physical Format: Print version:
Shilov, A.E. (Aleksandr Evgenʹevich), 1930-
Activation and catalytic reactions of saturated hydrocarbons in the presence of metal complexes.
Dordrecht ; Boston : Kluwer Academic Publishers, 2000
(DLC) 99054203
Material Type: Document, Internet resource
Document Type: Internet Resource, Computer File
All Authors / Contributors: A E Shilov; G B Shulʹpin
ISBN: 0792361016 9780792361015 661020487X 0306469456 9780306469459 9786610204878
OCLC Number: 133158551
Description: 1 online resource.
Contents: Cover --
Table of Contents --
Preface --
Introduction --
Chapter I. Processes of C ... H Bond Activation --
I.1. Chemical Reactivity of Hydrocarbons --
I.2. Cleavage of the C ... H Bond Promoted by Metal Complexes --
I.3. Brief History of Metal-Complex Activation of C ... H Bonds --
References --
Chapter II. Hydrocarbon Transformations That Do Not Involve Metals or Their Compounds --
II.1. Transformations Under the Action of Heat or Irradiation --
II.2. Reactions with Atoms, Free Radicals and Carbenes --
II.3. Oxidation by Molecular Oxygen --
II.4. Oxidation with Oxygen-containing Compounds --
II.5. Carboxylation --
II.6. Electrophilic Substitution of Hydrogen in Alkanes --
References --
Chapter III. Heterogeneous Hydrocarbon Reactions with Participation of Solid Metals and Metal Oxides --
III.1. Mechanisms of the Interaction between Alkanes and Catalyst Surfaces --
III.2. Isotope Exchange --
III.3. Isomerization --
III.4. Dehydrogenation and Dehydrocyclization --
III.5. Hydrogenolysis --
III.6. Heterogeneous Oxidation --
III.7. Oxidative and Nonoxidative Condensation of Alkanes --
III.8. Functionalization of C ... H Compounds --
References --
Chapter IV. Activation of C ... H Bonds by Low-Valent Metal Complexes ("the Organometallic Chemistry") --
IV. I. Formation of s-Organyl Hydride Complexes --
IV.2. Replacing Hydrogen Atoms by Various Groups --
IV. 3. Functionalization of C ... H Bonds with Intermediate Formation of Radicals and Carbenes --
IV.4. Cleavage of Some Other Bonds --
References --
Chapter V. Hydrocarbon Activation by Metal Ions, Atoms, and Complexes in the Gas Phase and in a Matrix --
V.1. Reactions with Metal Ions, Atoms, and Complexes in the Gas Phase --
V.2. Reactions with Metal Atoms in a Matrix --
References --
Chapter VI. Mechanisms of C-H Bond Splitting by Low-Valent Metal Complexes --
VI.1. Weak Coordination of Metal Ions with H ... H and C ... H Bonds --
VI.2. Mechanistic Studies --
VI.3. Thermodynamics of Oxidative Addition --
VI.4. Quantum-Chemical Calculations --
References --
Chapter VII. Activation of Hydrocarbons by Platinum Complexes --
VII.1. Non-Oxidative Reactions in the Presence of Pt(II) --
VII.2. Oxidation of Alkanes by Pt(IV) in the Presence of Pt(II) --
VII.3. Activation of Some Other C ... H Compounds --
VII.4. Photochemical Reactions of PtCl62- with Alkanes --
VII.5. On the Mechanism of Alkane Activation --
VII.6.s -Aryl Complexes of Pt(IV) Formed in Thermal and Photochemical Reactions of Aromatic Hydrocarbons with Pt(IV) Halide Com --
References --
CHAPTER VIII. Hydrocarbon Reactions with High-Valent Metal Complexes --
VIII.1. Electrophilic Metalation of C ... H Bonds ("Organometallic Activation") --
VIII.2. Oxidation in Aqueous and Acidic Media Promoted by Metal Cations and Complexes --
VIII.3. Oxidations by Metal Oxo Complexes --
VIII.4. Oxygenation by Peroxo Complexes --
References --
Chapter IX. Homogeneous Catalytic Oxidation of Hydrocarbons by Molecular Oxygen --
IX.1. Transition Metal Complexes in the Thermal Autoxidation of Hydrocarbons --
IX.2. Coupled Oxidation of Hydrocarbons --
IX.3. Photoinduced Metal-Catalyzed Oxidation of Hydrocarbons by Air --
References --
Chapter X. Homogeneous Catalytic Oxidation of Hydrocarbons by Peroxides and Other Oxygen Atom Donors --
X.1. Oxidation by Hydrogen Peroxide --
X.2. Ox.
Series Title: Catalysis by metal complexes, v. 21.
Responsibility: by Alexander E. Shilov and Georgy B. Shul'pin.

Abstract:

Among hydrocarbons, saturated hydrocarbons, alkanes (methane, ethane, propane, hexane etc. Saturated hydrocarbons may be called the "noble gases of organic chemistry" and, if so, the first  Read more...

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