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Thermodynamic and Kinetic Aspects of the Vitreous State

Author: S V Nemilov
Publisher: Milton : CRC Press, 2018.
Edition/Format:   eBook : Document : EnglishView all editions and formats
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Genre/Form: Electronic books
Additional Physical Format: Print version:
Nemilov, S.V.
Thermodynamic and Kinetic Aspects of the Vitreous State
Milton : CRC Press,c2018
Material Type: Document, Internet resource
Document Type: Internet Resource, Computer File
All Authors / Contributors: S V Nemilov
ISBN: 9781351094184 1351094181 9781351077286 1351077287
OCLC Number: 1020630085
Notes: Description based upon print version of record.
2. The Relation Between Relaxation Functions and the Prigogine-Defay Ratio
Description: 1 online resource (220 p.)
Contents: Cover; Half Title; Title Page; Copyright Page; Dedication; Table of Contents; Introduction; I. Origin of Glass: Thermodynamic Approximation; A. Thermodynamic Functions and Thermodynamic Variables; B. Classification of States According to Stability Features; C. Genesis of Nonequilibrium States of Liquid; D. Thermodynamic Model of the Vitreous State Genesis; 1. Basic Definitions and Assumptions of the Model; 2. Thermodynamics of the Glass Transition; E. Thermodynamic Criteria for the Glass Transition; II. Prigogine-Defay Ratio and the Problem of Structural Parameter Plurality A. Glass Transition as Compared to Phase Transitions of the First and Second OrderB. Thermodynamic Theory; C. Experiment; D. Simplest Models of Structural Parameters; E. General Models of Two Independent Structural Parameters; F. Basic Model Concepts of Glass Structure; G. Independent Parameters of Structure and the Silicate Melt Model; H. Experimental Evidence of Internal Changes Characteristic of Passing Through the Glass Transition Temperature; III. Thermodynamic Functions of Glasses; A. General Remarks; B. Kauzmannâ#x80;#x99;s Paradox; 1. The Essence of the Paradox; 2. Ways out of the Paradox C. Heat Capacity of Glasses and Empirical Correlations1. Quantum Theories of Heat Capacity; 2. Low-Temperature Anomaly of the Heat Capacity of Glasses; 3. Empirical Correlations; D. Relationship of the Reduced Thermodynamic Functions of Vitreous Systems: Thermodynamic Invariant of the Vitreous State; 1. Derivation of the Relation; 2. Analysis of the Relation; 3. Systematization of Glass Thermodynamic Functions (Thermodynamic Invariant of the Vitreous State); 4. Changing of Thermodynamic Functions as a Result of Annealing 5. Nonequilibrium State of Glass as a State of Unbalanced Interaction Potential Energy and Interacting Particlesâ#x80;#x99; Heat Energy6. Empirical Structural Correlations of the Zero-Point Entropy; 7. Peculiarities of Glassy Crystals: Components of Disorder Entropy; E. Glass as a System with Broken Ergodicity; 1. Specific Features of Nonergodicity in Glasses; 2. Basic Models Describing Glass Nonergodicity; 3. Principles of the Description of Glass as a Nonergodic System; IV. Order-Disorder Correlations in the Structure of Glass; A. Calculation of the Excess Entropy; 1. The Simplest Models 2. Topological ModelsB. Structural Reasons for the Excess Energy of Glasses; C. Inhomogeneity of Structure and Excess Thermodynamic Functions; D. Structural Investigations of the Ordering Character in Glasses; V. Thermodynamic Essence of Glass Structural Relaxation Processes; A. Adiabatic Relaxation; B. Isothermal Relaxation; C. Structural Relaxation and Density Fluctuations; D. The Memory Effect in Crossover Experiments; E. The Prigogine-Defay Ratio and the Relaxation Kinetics of Thermodynamic Properties; 1. Formal Aspect of the Description of Relaxation Kinetics

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