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Vacuum ultraviolet photoionization and photodissociation of molecules and clusters

Author: C Y Ng
Publisher: Singapore ; Teaneck, N.J. : World Scientific, ©1991.
Edition/Format:   eBook : Document : EnglishView all editions and formats
Summary:
This monograph reviews the recent progress in vacuum ultraviolet (VUV) photoionization and photodissociation processes. Photoionization, photoelectron, and fluorescence spectroscopic techniques have played an important role in revealing the photoionization and photodissociation dynamics of molecules in the vacuum ultraviolet region and in providing accurate energetic and spectroscopic information of ions as well as  Read more...
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Genre/Form: Electronic books
Additional Physical Format: Print version:
Vacuum ultraviolet photoionization and photodissociation of molecules and clusters.
Singapore ; Teaneck, N.J. : World Scientific, ©1991
(DLC) 91019621
(OCoLC)23868954
Material Type: Document, Internet resource
Document Type: Internet Resource, Computer File
All Authors / Contributors: C Y Ng
ISBN: 9789812814821 9812814825
OCLC Number: 828423968
Description: 1 online resource (viii, 572 pages) : illustrations
Contents: PREFACE; CONTENTS; PHOTOIONIZATION MASS SPECTROMETRIC STUDIES OF FREE RADICALS; I. INTRODUCTION; II. EXPERIMENTAL ARRANGEMENT; A. The Photoionization Mass Spectrometric Method; B. Generation of Transient Species for PIMS Studies; III. SURVEY OF EXPERIMENTAL RESULTS; A. The Pnicogen and Chalcogen Hydrides (Group V and VI Hydrides); B. The Nitrogen and Phosphorus Fluorides; C. The Group IV Hydrides; 1. The CHn, SiHn and GeHn Sequence; a. The SiHn System.; b. The GeHn System; 2. Comparisons of CHn, SiHn, GeHn; a. Step-wise Bond Energies; b. Jahn-Teller Distortion in CH4+, SiH4+, GeH4+ 3. C2H3 and C2H5: C-H Bond Energies of Ethylene and Ethane Some Observations on the C-H Bond Energy in Acetylene; D. The Boron Hydrides; 1. BH3; 2. B2H5; 3. B2H4; E. COOH --
an Important Reaction Intermediate; F. SO and P2; Some General Observations on Transient Species; IV. CONCLUDING REMARKS; Acknowledgment; References; PHOTOELECTRON SPECTROSCOPY OF SHORT-LIVED MOLECULES; I. INTRODUCTION; II. THE BACKGROUND; III. PES OF SHORT-LIVED MOLECULES GENERATED BY RAPID ATOM-MOLECULE REACTIONS. IV. A CASE STUDY: A PES STUDY OF THE 1-FLUOROETHYL AND 1,2-DIFLUOROETHYL RADICALS PREPARED BY FLUORINE-ATOM ABSTRACTION REACTIONSVI. 1. Introduction; VI. 2. Experiment; VI. 2.a. F + C2H5F; IV. 2.b. F + FCH2CH2F; IV. 3. The Hel Photoelectron Spectrum of 1,2-difluorethane; IV. 4. Computational Details; IV. 4.a. F + C2H5F; IV. 4.b. F + FCH2CH2F; IV. 5. Results and Discussion; IV. 5.a. F + C2H5F; IV. 5.b. F + FCH2CH2F; V. POSSIBLE DIRECTIONS FOR THE FUTURE; ACKNOWLEDGMENTS; REFERENCES; APPENDIX; PROTON TRANSFER IN IONIC STATES OF HYDROGEN-BONDED DIMERS. A PHOTOELECTRON SPECTROSCOPIC APPROACH. I. INTRODUCTIONII. EXPERIMENTAL AND THEORETICAL BACKGROUND; A. Supersonic Nozzle Beam Photoelectron Spectrometer; B. PES vs PIMS; C. Theoretical Method; D. Production and Concentration of Hydrogen-Bonded Dimers; E. Structures of Hydrogen-Bonded Dimers; 1. Water Dimer; 2. Ammonia Dimer; 3. Hydrogen Fluoride Dimer; 4. Formic Acid Dimer; 5. Methanol Dimer; III. PHOTOELECTRON SPECTRUM AND VERTICAL IONIZATION ENERGY; A. Water Dimer; B. Formic Acid Dimer; C. Methanol Dimer; D. Ammonia Dimer; IV. POTENTIAL ENERGY SURFACES OF WATER DIMER CATION; A. Modeling; B. Water Dimer. C. Proton-Transfer Potential-Energy SurfaceD. Ionization Energies of the Water Dimer; E. Adiabatic Ionization Energy; F. Equilibrium Geometry of Water Dimer Cation; G. Dissociation Energies of Water Dimer Cation; V. IONIZATIONS OF AMMONIA DIMER AND HF DIMER; A. PIMS Results of Ammonia Dimer; B. Structure and Potential Curves of (NH3)2 and (NH3)2+; 1. Ammonia Dimer; 2. Equilibrium Structure of Ammonia Dimer Cation; 3. Potential Energy Curves of Ammonia Dimer Cation; 4. Dissociation Energies of Ammonia Dimer Cation; C. Ionization Energies of Ammonia Dimer; D. Ionization of HF Dimer.
Responsibility: edited by C.Y. Ng.

Abstract:

This monograph reviews the recent progress in vacuum ultraviolet (VUV) photoionization and photodissociation processes. Photoionization, photoelectron, and fluorescence spectroscopic techniques have played an important role in revealing the photoionization and photodissociation dynamics of molecules in the vacuum ultraviolet region and in providing accurate energetic and spectroscopic information of ions as well as neutral molecules. The book represents the first detailed review of major experimental developments in the studies of single vacuum ultraviolet photon ionization and dissociation pr.

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