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LABORATORY INVESTIGATIONS IN SUPPORT OF FLUID BED FLUORIDE VOLATILITY PROCESSES. PART III. SEPARATION OF GASEOUS MIXTURES OF URANIUM HEXAFLUORIDE AND PLUTONIUM HEXAFLUORIDE BY THERMAL DECOMPOSITION. Preview this item
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LABORATORY INVESTIGATIONS IN SUPPORT OF FLUID BED FLUORIDE VOLATILITY PROCESSES. PART III. SEPARATION OF GASEOUS MIXTURES OF URANIUM HEXAFLUORIDE AND PLUTONIUM HEXAFLUORIDE BY THERMAL DECOMPOSITION.

Author: Trevorrow, L.; Fischer, J.; Riha, J.; Argonne National Laboratory.; United States. Department of Energy. Office of Scientific and Technical Information.
Publisher: Argonne, Ill. : Argonne National Laboratory ; Oak Ridge, Tenn. : distributed by the Office of Scientific and Technical Information, U.S. Dept. of Energy, [1963] [1963] 1963
Series: ANL (Series), 6762.
Edition/Format:   eBook : Document : National government publication : English
Summary:
Experiments were carried out to determine the extent and rate of separation of mixtures of uranium hexafluoride and plutonium hexafluoride by selective thermal decomposition. Gaseous mixtures of uranium hexafluoride, plutonium hexafluoride, and helium were circulated for varying lengths of time through nickel vessels packed with nickel wool at temperatures of 150, 200, and 300 deg C. The initial ratios of uranium  Read more...
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Additional Physical Format: Print version:
Trevorrow, L.
Laboratory investigations in support of fluid bed fluoride volatility processes. Part III, Separation of gaseous mixtures of uranium hexafluoride and plutonium hexafluoride by thermal decomposition.
Lemont, III. : Argonne National Laboratory, 1963
(OCoLC)263869718
Material Type: Document, Government publication, National government publication, Internet resource
Document Type: Internet Resource, Computer File
All Authors / Contributors: Trevorrow, L.; Fischer, J.; Riha, J.; Argonne National Laboratory.; United States. Department of Energy. Office of Scientific and Technical Information.
OCLC Number: 1065872427
Notes: Published through SciTech Connect.
08/01/1963.
"anl-6762"
Trevorrow, L.; Fischer, J.; Riha, J.
Reproduction Notes: Electronic reproduction. [S.l.] : HathiTrust Digital Library, 2010. MiAaHDL
Description: 1 online resource (Pages: 15 :) PDF file.
Details: Master and use copy. Digital master created according to Benchmark for Faithful Digital Reproductions of Monographs and Serials, Version 1. Digital Library Federation, December 2002.
Series Title: ANL (Series), 6762.

Abstract:

Experiments were carried out to determine the extent and rate of separation of mixtures of uranium hexafluoride and plutonium hexafluoride by selective thermal decomposition. Gaseous mixtures of uranium hexafluoride, plutonium hexafluoride, and helium were circulated for varying lengths of time through nickel vessels packed with nickel wool at temperatures of 150, 200, and 300 deg C. The initial ratios of uranium hexafluoride to plutonium hexafluoride in the mixtures were of the order of 10 to 1. The gas phase was analyzed for uranium and plutonium before and after circulation. The amounts of uranium and plutonium in the solid compounds deposited in the vessels were also determined. Passage of the mixtures through the hot vessels resulted in the removal of 99.5 to 99.9% of the plutonium. The solid product remaining in the vessels was plutonium tetrafluoride containing 0.09 to 1.3% uranium. The separation of plutonium hexafluoride from uranium hexafluoride by selective thermal decomposition is applicable to fluid bed fluoride volatility processes for the recovery of fissile material from reactor fuels. (auth).

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