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Propriétés de transport des sels de lithium LiTDI et LiFSI : application à la formulation d'électrolytes optimisés pour batteries Li-ion

Author: Christopher Logan BerhautMeriem Anouti-BenaichoucheDaniel LemordantMichel Rosso, chercheur en physique).Patrick JudeinsteinAll authors
Publisher: 2016.
Dissertation: Thèse de doctorat : Chimie-Physique, spécialité électrochimie : Tours : 2016.
Edition/Format:   Computer file : Document : Thesis/dissertation : French
Summary:
La plupart des batteries Li-ion aujourd'hui utilisent des électrolytes à base de LiPF6 un sel de lithium connu pour son instabilité chimique au-delà de 60°C car il se dégrade en libérant PF5 et LiF. En présence de traces d'eau il génère en plus des composés oxyfluorophosphorés et du HF qui peut être dommageable à la fois pour les performances et pour le vieillissement de l'accumulateur. Plusieurs sels
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Genre/Form: Thèses et écrits académiques
Material Type: Document, Thesis/dissertation, Internet resource
Document Type: Internet Resource, Computer File
All Authors / Contributors: Christopher Logan Berhaut; Meriem Anouti-Benaichouche; Daniel Lemordant; Michel Rosso, chercheur en physique).; Patrick Judeinstein; Pascal Mailley; Laure Timperman; Patrick Bernard; Université de Tours.; École doctorale Énergie, Matériaux, Sciences de la Terre et de l'Univers (Centre-Val de Loire).; Physico-Chimie des Matériaux et des Électrolytes pour l'Énergie (Tours).
OCLC Number: 973888883
Notes: Titre provenant de l'écran-titre.
Description: 1 online resource
Responsibility: Christopher Logan Berhaut ; sous la direction de Meriem Anouti-Benaichouche et de Daniel Lemordant.

Abstract:

La plupart des batteries Li-ion aujourd'hui utilisent des électrolytes à base de LiPF6 un sel de lithium connu pour son instabilité chimique au-delà de 60°C car il se dégrade en libérant PF5 et LiF. En présence de traces d'eau il génère en plus des composés oxyfluorophosphorés et du HF qui peut être dommageable à la fois pour les performances et pour le vieillissement de l'accumulateur. Plusieurs sels sont candidats au remplacement de LiPF6, notamment ceux basés sur les anions fluorosulfonylamidures et les anions de Hückel. Ce travail concerne l'étude des propriétés physico-chimiques et de transport des électrolytes à base de 4,5-dicyano-2- (trifluoromethyl)imidazolide de lithium (LiTDI) et bis(fluorosulfonyl)amidure de lithium (LiFSI) pour une utilisation au sein d'accumulateurs de type Li-ion. Dans ce travail il a d'abord été montré que LiTDI n'est que faiblement dissocié dans les mélanges de carbonates d'alkyles utilisés dans les batteries Li-ion tels que le binaire (EC/DMC) ce qui limite sa conductivité. Pour pouvoir remédier à cet inconvénient, une étude des phénomènes de solvatation et d'associations ioniques a été menée et a conduit à proposer un mélange ternaire de solvants (EC/GBL/MP) dans lequel LiTDI est plus dissocié. Le mélange ternaire proposé améliore à la fois les propriétés de transport et les caractéristiques thermiques de l'électrolyte sans compromettre le domaine de stabilité chimique et électrochimique. Enfin, le nouvel électrolyte EC/GBL/MP contenant LiTDI, a été testé en accumulateurs dans les conditions opératoires usuelles (régime C/10 et température ambiante) et sévères (régime 10C et des températures allant de -20 °C à 60 °C). Le problème de corrosion de l'aluminium de LiFSI a aussi été pris en compte. Un électrolyte prometteur à base d'un mélange LiTDI/LiFSI montrant de meilleures performances que chaque sel utilisé séparément dans EC/DMC a été présenté. Les conclusions de cette thèse prouvent que LiTDI ou LiFSI peuvent être utilisés comme sels de lithium dans les électrolytes pour accumulateurs Li-ion.

Most of the Li-ion batteries used in electrical devices contain a solution of LiPF6 in alkylcarbonate solvents with the risk of releasing PF5 at elevated temperatures and HF in the presence of water. Several salts are candidates for the replacement of LiPF6, including those based on fluorosulfonylamides and Hückel anions. This work concerns the study of physicochemical and transport properties of lithium 4,5-dicyano-2- (trifluoromethyl)imidazolide (LiTDI) and lithium bis(fluorosulfonyl)amide (LiFSI) based electrolytes and their use in Li-ion battery. First it was revealed that LiTDI is only weakly dissociated in alkylcarbonate mixtures used in Li-ion batteries such as EC/DMC limiting its conductivity. To overcome this disadvantage, a study of the solvation phenomena and of ionic association within the electrolytes was conducted. This study led to a ternary mixture of solvents (EC/GBL/MP) in which LiTDI is more dissociated. This new solvent mixture improves both the transport properties and the thermal stability of the LiTDI based electrolyte without compromising its chemical and electrochemical stability. Finally, the new LiTDI in EC/GBL/MP electrolyte was tested in NMC/graphite batteries under normal (C/10 rate and room temperature) and severe (10C rate and temperatures varying from - 20 ° C to 60 °C) operating conditions. The aluminium corrosion problem encountered by LiFSI based electrolytes was taken into account and a LiTDI/LiFSI salt mixture based electrolyte showing promising results was presented. The findings of this thesis show that LiTDI or LiFSI can be used as lithium salts in electrolytes for Li-ion batteries.

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<http:\/\/www.worldcat.org\/oclc\/973888883<\/a>> # Propri\u00E9t\u00E9s de transport des sels de lithium LiTDI et LiFSI : application \u00E0 la formulation d\'\u00E9lectrolytes optimis\u00E9s pour batteries Li-ion<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:CreativeWork<\/a>, schema:MediaObject<\/a>, bgn:ComputerFile<\/a>, bgn:Thesis<\/a> ;\u00A0\u00A0\u00A0\nbgn:inSupportOf<\/a> \"Th\u00E8se de doctorat : Chimie-Physique, sp\u00E9cialit\u00E9 \u00E9lectrochimie : Tours : 2016.<\/span>\" ;\u00A0\u00A0\u00A0\nlibrary:oclcnum<\/a> \"973888883<\/span>\" ;\u00A0\u00A0\u00A0\nlibrary:placeOfPublication<\/a> <http:\/\/id.loc.gov\/vocabulary\/countries\/fr<\/a>> ;\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/electrolytes_stabilite<\/a>> ; # \u00C9lectrolytes--Stabilit\u00E9<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/accumulateurs_au_lithium<\/a>> ; # Accumulateurs au lithium<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/anions<\/a>> ; # Anions<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/resistance_des_materiaux<\/a>> ; # R\u00E9sistance des mat\u00E9riaux<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/litdi<\/a>> ; # LiTDI<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/batterie_lithium_ion<\/a>> ; # Batterie lithium-ion<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/lifsi<\/a>> ; # LiFSI<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/sei<\/a>> ; # SEI<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/conduction_ionique<\/a>> ; # Conduction ionique<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/solvant_effets_de_chimie<\/a>> ; # Solvant, Effets de (chimie)<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/graphite<\/a>> ; # Graphite<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/sel_de_lithium<\/a>> ; # Sel de lithium<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/sels_de_lithium<\/a>> ; # Sels de lithium<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/electrode_nmc<\/a>> ; # \u00C9lectrode NMC<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/electrolyte<\/a>> ; # \u00C9lectrolyte<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/propriete_de_transport<\/a>> ; # Propri\u00E9t\u00E9 de transport<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/interfaces<\/a>> ; # Interfaces<\/span>\n\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/solvatation<\/a>> ; # Solvatation<\/span>\n\u00A0\u00A0\u00A0\nschema:author<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/berhaut_christopher_logan_1989<\/a>> ; # Christopher Logan Berhaut<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/universite_de_tours<\/a>> ; # Universit\u00E9 de Tours.<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/timperman_laure_1984<\/a>> ; # Laure Timperman<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/bernard_patrick<\/a>> ; # Patrick Bernard<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/ecole_doctorale_energie_materiaux_sciences_de_la_terre_et_de_l_univers_centre_val_de_loire<\/a>> ; # \u00C9cole doctorale \u00C9nergie, Mat\u00E9riaux, Sciences de la Terre et de l\'Univers (Centre-Val de Loire).<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/physico_chimie_des_materiaux_et_des_electrolytes_pour_l_energie_tours<\/a>> ; # Physico-Chimie des Mat\u00E9riaux et des \u00C9lectrolytes pour l\'\u00C9nergie (Tours).<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/judeinstein_patrick<\/a>> ; # Patrick Judeinstein<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/rosso_michel_19_chercheur_en_physique<\/a>> ; # chercheur en physique). Michel Rosso<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/lemordant_daniel_1946<\/a>> ; # Daniel Lemordant<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/anouti_benaichouche_meriem_1965<\/a>> ; # Meriem Anouti-Benaichouche<\/span>\n\u00A0\u00A0\u00A0\nschema:contributor<\/a> <http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/mailley_pascal<\/a>> ; # Pascal Mailley<\/span>\n\u00A0\u00A0\u00A0\nschema:datePublished<\/a> \"2016<\/span>\" ;\u00A0\u00A0\u00A0\nschema:description<\/a> \"La plupart des batteries Li-ion aujourd\'hui utilisent des \u00E9lectrolytes \u00E0 base de LiPF6 un sel de lithium connu pour son instabilit\u00E9 chimique au-del\u00E0 de 60\u00B0C car il se d\u00E9grade en lib\u00E9rant PF5 et LiF. En pr\u00E9sence de traces d\'eau il g\u00E9n\u00E8re en plus des compos\u00E9s oxyfluorophosphor\u00E9s et du HF qui peut \u00EAtre dommageable \u00E0 la fois pour les performances et pour le vieillissement de l\'accumulateur. Plusieurs sels sont candidats au remplacement de LiPF6, notamment ceux bas\u00E9s sur les anions fluorosulfonylamidures et les anions de H\u00FCckel. Ce travail concerne l\'\u00E9tude des propri\u00E9t\u00E9s physico-chimiques et de transport des \u00E9lectrolytes \u00E0 base de 4,5-dicyano-2- (trifluoromethyl)imidazolide de lithium (LiTDI) et bis(fluorosulfonyl)amidure de lithium (LiFSI) pour une utilisation au sein d\'accumulateurs de type Li-ion. Dans ce travail il a d\'abord \u00E9t\u00E9 montr\u00E9 que LiTDI n\'est que faiblement dissoci\u00E9 dans les m\u00E9langes de carbonates d\'alkyles utilis\u00E9s dans les batteries Li-ion tels que le binaire (EC\/DMC) ce qui limite sa conductivit\u00E9. Pour pouvoir rem\u00E9dier \u00E0 cet inconv\u00E9nient, une \u00E9tude des ph\u00E9nom\u00E8nes de solvatation et d\'associations ioniques a \u00E9t\u00E9 men\u00E9e et a conduit \u00E0 proposer un m\u00E9lange ternaire de solvants (EC\/GBL\/MP) dans lequel LiTDI est plus dissoci\u00E9. Le m\u00E9lange ternaire propos\u00E9 am\u00E9liore \u00E0 la fois les propri\u00E9t\u00E9s de transport et les caract\u00E9ristiques thermiques de l\'\u00E9lectrolyte sans compromettre le domaine de stabilit\u00E9 chimique et \u00E9lectrochimique. Enfin, le nouvel \u00E9lectrolyte EC\/GBL\/MP contenant LiTDI, a \u00E9t\u00E9 test\u00E9 en accumulateurs dans les conditions op\u00E9ratoires usuelles (r\u00E9gime C\/10 et temp\u00E9rature ambiante) et s\u00E9v\u00E8res (r\u00E9gime 10C et des temp\u00E9ratures allant de -20 \u00B0C \u00E0 60 \u00B0C). Le probl\u00E8me de corrosion de l\'aluminium de LiFSI a aussi \u00E9t\u00E9 pris en compte. Un \u00E9lectrolyte prometteur \u00E0 base d\'un m\u00E9lange LiTDI\/LiFSI montrant de meilleures performances que chaque sel utilis\u00E9 s\u00E9par\u00E9ment dans EC\/DMC a \u00E9t\u00E9 pr\u00E9sent\u00E9. Les conclusions de cette th\u00E8se prouvent que LiTDI ou LiFSI peuvent \u00EAtre utilis\u00E9s comme sels de lithium dans les \u00E9lectrolytes pour accumulateurs Li-ion.<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\nschema:description<\/a> \"Most of the Li-ion batteries used in electrical devices contain a solution of LiPF6 in alkylcarbonate solvents with the risk of releasing PF5 at elevated temperatures and HF in the presence of water. Several salts are candidates for the replacement of LiPF6, including those based on fluorosulfonylamides and H\u00FCckel anions. This work concerns the study of physicochemical and transport properties of lithium 4,5-dicyano-2- (trifluoromethyl)imidazolide (LiTDI) and lithium bis(fluorosulfonyl)amide (LiFSI) based electrolytes and their use in Li-ion battery. First it was revealed that LiTDI is only weakly dissociated in alkylcarbonate mixtures used in Li-ion batteries such as EC\/DMC limiting its conductivity. To overcome this disadvantage, a study of the solvation phenomena and of ionic association within the electrolytes was conducted. This study led to a ternary mixture of solvents (EC\/GBL\/MP) in which LiTDI is more dissociated. This new solvent mixture improves both the transport properties and the thermal stability of the LiTDI based electrolyte without compromising its chemical and electrochemical stability. Finally, the new LiTDI in EC\/GBL\/MP electrolyte was tested in NMC\/graphite batteries under normal (C\/10 rate and room temperature) and severe (10C rate and temperatures varying from - 20 \u00B0 C to 60 \u00B0C) operating conditions. The aluminium corrosion problem encountered by LiFSI based electrolytes was taken into account and a LiTDI\/LiFSI salt mixture based electrolyte showing promising results was presented. The findings of this thesis show that LiTDI or LiFSI can be used as lithium salts in electrolytes for Li-ion batteries.<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\nschema:exampleOfWork<\/a> <http:\/\/worldcat.org\/entity\/work\/id\/4083721269<\/a>> ;\u00A0\u00A0\u00A0\nschema:genre<\/a> \"Th\u00E8ses et \u00E9crits acad\u00E9miques<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\nschema:inLanguage<\/a> \"fr<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Propri\u00E9t\u00E9s de transport des sels de lithium LiTDI et LiFSI : application \u00E0 la formulation d\'\u00E9lectrolytes optimis\u00E9s pour batteries Li-ion<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\nschema:productID<\/a> \"973888883<\/span>\" ;\u00A0\u00A0\u00A0\nschema:url<\/a> <http:\/\/theses.scd.univ-tours.fr\/index.php?fichier=2016\/christopher.berhaut_6783.pdf<\/a>> ;\u00A0\u00A0\u00A0\nschema:url<\/a> <http:\/\/www.theses.fr\/2016TOUR4017\/document<\/a>> ;\u00A0\u00A0\u00A0\nwdrs:describedby<\/a> <http:\/\/www.worldcat.org\/title\/-\/oclc\/973888883<\/a>> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n\n

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<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/ecole_doctorale_energie_materiaux_sciences_de_la_terre_et_de_l_univers_centre_val_de_loire<\/a>> # \u00C9cole doctorale \u00C9nergie, Mat\u00E9riaux, Sciences de la Terre et de l\'Univers (Centre-Val de Loire).<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Organization<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"\u00C9cole doctorale \u00C9nergie, Mat\u00E9riaux, Sciences de la Terre et de l\'Univers (Centre-Val de Loire).<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/physico_chimie_des_materiaux_et_des_electrolytes_pour_l_energie_tours<\/a>> # Physico-Chimie des Mat\u00E9riaux et des \u00C9lectrolytes pour l\'\u00C9nergie (Tours).<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Organization<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Physico-Chimie des Mat\u00E9riaux et des \u00C9lectrolytes pour l\'\u00C9nergie (Tours).<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Organization\/universite_de_tours<\/a>> # Universit\u00E9 de Tours.<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Organization<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Universit\u00E9 de Tours.<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/anouti_benaichouche_meriem_1965<\/a>> # Meriem Anouti-Benaichouche<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:birthDate<\/a> \"1965<\/span>\" ;\u00A0\u00A0\u00A0\nschema:deathDate<\/a> \"\" ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Anouti-Benaichouche<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Meriem<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Meriem Anouti-Benaichouche<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/berhaut_christopher_logan_1989<\/a>> # Christopher Logan Berhaut<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:birthDate<\/a> \"1989<\/span>\" ;\u00A0\u00A0\u00A0\nschema:deathDate<\/a> \"\" ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Berhaut<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Christopher Logan<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Christopher Logan Berhaut<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/bernard_patrick<\/a>> # Patrick Bernard<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Bernard<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Patrick<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Patrick Bernard<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/judeinstein_patrick<\/a>> # Patrick Judeinstein<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Judeinstein<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Patrick<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Patrick Judeinstein<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/lemordant_daniel_1946<\/a>> # Daniel Lemordant<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:birthDate<\/a> \"1946<\/span>\" ;\u00A0\u00A0\u00A0\nschema:deathDate<\/a> \"\" ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Lemordant<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Daniel<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Daniel Lemordant<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/mailley_pascal<\/a>> # Pascal Mailley<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Mailley<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Pascal<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Pascal Mailley<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/rosso_michel_19_chercheur_en_physique<\/a>> # chercheur en physique). Michel Rosso<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:birthDate<\/a> \"19..<\/span>\" ;\u00A0\u00A0\u00A0\nschema:deathDate<\/a> \";<\/span>\" ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Rosso<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Michel<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"chercheur en physique). Michel Rosso<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Person\/timperman_laure_1984<\/a>> # Laure Timperman<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Person<\/a> ;\u00A0\u00A0\u00A0\nschema:birthDate<\/a> \"1984<\/span>\" ;\u00A0\u00A0\u00A0\nschema:deathDate<\/a> \"\" ;\u00A0\u00A0\u00A0\nschema:familyName<\/a> \"Timperman<\/span>\" ;\u00A0\u00A0\u00A0\nschema:givenName<\/a> \"Laure<\/span>\" ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Laure Timperman<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/batterie_lithium_ion<\/a>> # Batterie lithium-ion<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Batterie lithium-ion<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/electrode_nmc<\/a>> # \u00C9lectrode NMC<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"\u00C9lectrode NMC<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/electrolyte<\/a>> # \u00C9lectrolyte<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"\u00C9lectrolyte<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/graphite<\/a>> # Graphite<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Graphite<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/interfaces<\/a>> # Interfaces<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Interfaces<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/lifsi<\/a>> # LiFSI<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"LiFSI<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/litdi<\/a>> # LiTDI<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"LiTDI<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/propriete_de_transport<\/a>> # Propri\u00E9t\u00E9 de transport<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Propri\u00E9t\u00E9 de transport<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/sei<\/a>> # SEI<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"SEI<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Thing\/sel_de_lithium<\/a>> # Sel de lithium<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Thing<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Sel de lithium<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/accumulateurs_au_lithium<\/a>> # Accumulateurs au lithium<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Accumulateurs au lithium<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/anions<\/a>> # Anions<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Anions<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/conduction_ionique<\/a>> # Conduction ionique<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Conduction ionique<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/electrolytes_stabilite<\/a>> # \u00C9lectrolytes--Stabilit\u00E9<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"\u00C9lectrolytes--Stabilit\u00E9<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/resistance_des_materiaux<\/a>> # R\u00E9sistance des mat\u00E9riaux<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"R\u00E9sistance des mat\u00E9riaux<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/sels_de_lithium<\/a>> # Sels de lithium<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Sels de lithium<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/solvant_effets_de_chimie<\/a>> # Solvant, Effets de (chimie)<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Solvant, Effets de (chimie)<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/experiment.worldcat.org\/entity\/work\/data\/4083721269#Topic\/solvatation<\/a>> # Solvatation<\/span>\n\u00A0\u00A0\u00A0\u00A0a \nschema:Intangible<\/a> ;\u00A0\u00A0\u00A0\nschema:name<\/a> \"Solvatation<\/span>\"@fr<\/a> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/id.loc.gov\/vocabulary\/countries\/fr<\/a>>\u00A0\u00A0\u00A0\u00A0a \nschema:Place<\/a> ;\u00A0\u00A0\u00A0\ndcterms:identifier<\/a> \"fr<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/www.theses.fr\/2016TOUR4017\/document<\/a>>\u00A0\u00A0\u00A0\nrdfs:comment<\/a> \"Acc\u00E8s au texte int\u00E9gral<\/span>\" ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n
<http:\/\/www.worldcat.org\/title\/-\/oclc\/973888883<\/a>>\u00A0\u00A0\u00A0\u00A0a \ngenont:InformationResource<\/a>, genont:ContentTypeGenericResource<\/a> ;\u00A0\u00A0\u00A0\nschema:about<\/a> <http:\/\/www.worldcat.org\/oclc\/973888883<\/a>> ; # Propri\u00E9t\u00E9s de transport des sels de lithium LiTDI et LiFSI : application \u00E0 la formulation d\'\u00E9lectrolytes optimis\u00E9s pour batteries Li-ion<\/span>\n\u00A0\u00A0\u00A0\nschema:dateModified<\/a> \"2021-02-17<\/span>\" ;\u00A0\u00A0\u00A0\nvoid:inDataset<\/a> <http:\/\/purl.oclc.org\/dataset\/WorldCat<\/a>> ;\u00A0\u00A0\u00A0\u00A0.\n\n\n<\/div>\n\n

Content-negotiable representations<\/p>\n